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Solar-driven interfacial evaporation technologies for food, energy and water
Solar-driven interfacial evaporation technologies use solar energy to heat materials that drive water evaporation. These technologies are versatile and do not require electricity, which enables their potential application across the food, energy and water nexus. In this Review, we assess the potential of solar-driven interfacial evaporation technologies in food, energy and clean-water production, in wastewater treatment, and in resource recovery. Interfacial evaporation technologies can produce up to 5.3 l m–2 h−1 of drinking water using sunlight as the energy source. Systems designed for food production in coastal regions desalinate water to irrigate crops or wash contaminated soils. Technologies are being developed to simultaneously produce both clean energy and water through interfacial evaporation and have reached up to 204 W m–2 for electricity and 2.5 l m–2 h–1 for water in separate systems. Other solar evaporation approaches or combinations of approaches could potentially use the full solar spectrum to generate multiple products (such as water, food, electricity, heating or cooling, and/or fuels). In the future, solar evaporation technologies could aid in food, energy and water provision in low-resource or rural settings that lack reliable access to these essentials, but the systems must first undergo rigorous, scaled-up field testing to understand their performance, stability and competitiveness.
Higher temperature sensitivity of forest soil methane oxidation in colder climates
Forest soils, serving as an important sink for atmospheric methane (CH4), modulate the global CH4 budget. However, the direction and magnitude of the forest soil CH4 sink under warming remain uncertain, partly because the temperature response of microbial CH4 oxidation varies substantially across geographical scales. Here, we reveal the spatial variation in the response of forest soil microbial CH4 oxidation to warming, along with the driving factors, across 84 sites spanning a broad latitudinal gradient in eastern China. Our results show that the temperature sensitivity of soil microbial CH4 oxidation significantly declines with increasing site mean annual temperature, with a range of 0.03 to 0.77 μg CH4 g–1 soil d–1 °C–1. Moreover, soil resources and type II methanotrophs play crucial roles in shaping the temperature sensitivity of soil microbial CH4 oxidation. Our findings highlight the importance of incorporating climate, soil resources, and methanotroph groups into biogeochemical models to more realistically predict forest soil CH4 sink under warming.
Photo-assisted technologies for environmental remediation
Industrial processes can lead to air and water pollution, particularly from organic contaminants such as toluene and antibiotics, posing threats to human health. Photo-assisted chemical oxidation technologies leverage light energy to mineralize these contaminants. In this Review, we discuss the mechanisms and efficiencies of photo-assisted advanced oxidation processes for wastewater treatment and photothermal technologies for air purification. The integration of solar energy enhances degradation efficiency and reduces energy consumption, enabling more efficient remediation methods. We evaluate the technological aspects of photo-assisted technologies, such as photo-Fenton, photo-persulfate activation, photo-ozonation and photoelectrochemical oxidation, emphasizing their potential for practical applications. Finally, we discuss the challenges in scaling up photo-assisted technologies for specific environmental remediation needs. Photo-assisted technologies have demonstrated effectiveness in environmental remediation, although large-scale applications remain constrained by high costs. Future potential applications of photo-assisted technologies will require that technology selection be tailored to specific pollution scenarios and engineering processes optimized to minimize costs.
Impact of transboundary water flows on quality-induced water pressure in China
Quality-induced water pressure (P) is gaining increased attention. With the flows of transboundary water, P can be transferred among upstream and downstream regions. Here, we quantified the magnitude of pollutant transmission, and assessed its impact on individual provinces in China. On the annual basis, P was mitigated in 61% of provinces for Chemical Oxygen Demand, 87% for Ammonia Nitrogen, and 84% for Total Phosphorus, while it was intensified for 77% for Total Nitrogen in 2021. The aggregated P were mitigated in 68% of provinces, while intensified in 32% provinces. Furthermore, the monthly assessment has found that the impact of transboundary water on P varies seasonally, generally alleviating in winter and exacerbating in summer. This fluctuation was attributed to the comparatively higher quality of transboundary inflows during winter relative to local water quality. This study provides a scientific foundation for effective water management and quality control.
Anthropogenic organic aerosol in Europe produced mainly through second-generation oxidation
Exposure to anthropogenic atmospheric aerosol is a major health issue, causing several million deaths per year worldwide. The oxidation of aromatic hydrocarbons from traffic and wood combustion is an important anthropogenic source of low-volatility species in secondary organic aerosol, especially in heavily polluted environments. It is not yet established whether the formation of anthropogenic secondary organic aerosol involves mainly rapid autoxidation, slower sequential oxidation steps or a combination of the two. Here we reproduced a typical urban haze in the ‘Cosmics Leaving Outdoor Droplets’ chamber at the European Organization for Nuclear Research and observed the dynamics of aromatic oxidation products during secondary organic aerosol growth on a molecular level to determine mechanisms underlying their production and removal. We demonstrate that sequential oxidation is required for substantial secondary organic aerosol formation. Second-generation oxidation decreases the products’ saturation vapour pressure by several orders of magnitude and increases the aromatic secondary organic aerosol yields from a few percent to a few tens of percent at typical atmospheric concentrations. Through regional modelling, we show that more than 70% of the exposure to anthropogenic organic aerosol in Europe arises from second-generation oxidation.
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