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A hybrid single quantum dot coupled cavity on a CMOS-compatible SiC photonic chip for Purcell-enhanced deterministic single-photon emission
The ability to control nonclassical light emission from a single quantum emitter by an integrated cavity may unleash new perspectives for integrated photonic quantum applications. However, coupling a single quantum emitter to cavity within photonic circuitry towards creation of the Purcell-enhanced single-photon emission is elusive due to the complexity of integrating active devices in low-loss photonic circuits. Here we demonstrate a hybrid micro-ring resonator (HMRR) coupled with self-assembled quantum dots (QDs) for cavity-enhanced deterministic single-photon emission. The HMRR cavity supports whispering-gallery modes with quality factors up to 7.8×103. By further introducing a micro-heater, we show that the photon emission of QDs can be locally and dynamically tuned over one free spectral ranges of the HMRR ( ~ 4 nm). This allows precise tuning of individual QDs in resonance with the cavity modes, thereby enhancing single-photon emission with a Purcell factor of about 4.9. Our results on the hybrid integrated cavities coupled with two-level quantum emitters emerge as promising devices for chip-based scalable photonic quantum applications.
Ultrafast pump-probe phase-randomized tomography
Measuring fluctuations in matter’s low-energy excitations is the key to unveiling the nature of the non-equilibrium response of materials. A promising outlook in this respect is offered by spectroscopic methods that address matter fluctuations by exploiting the statistical nature of light-matter interactions with weak few-photon probes. Here we report the first implementation of ultrafast phase randomized tomography, combining pump-probe experiments with quantum optical state tomography, to measure the ultrafast non-equilibrium dynamics in complex materials. Our approach utilizes a time-resolved multimode heterodyne detection scheme with phase-randomized coherent ultrashort laser pulses, overcoming the limitations of phase-stable configurations and enabling a robust reconstruction of the statistical distribution of phase-averaged optical observables. This methodology is validated by measuring the coherent phonon response in α-quartz. By tracking the dynamics of the shot-noise limited photon number distribution of few-photon probes with ultrafast resolution, our results set an upper limit to the non-classical features of phononic state in α-quartz and provide a pathway to access non-equilibrium quantum fluctuations in more complex quantum materials.
Programmable electron-induced color router array
The development of color routers (CRs) realizes the splitting of dichromatic components, contributing to the modulation of photon momentum that acts as the information carrier for optical information technology on the frequency and spatial domains. However, CRs with optical stimulation lack active control of photon momentum at deep subwavelength scale because of the optical diffraction limit. Here, we experimentally demonstrate an active manipulation of dichromatic photon momentum at a deep subwavelength scale via electron-induced CRs, where the CRs radiation patterns are manipulated by steering the electron impact position within 60 nm in a single nanoantenna unit. Moreover, an encrypted display device based on programmable modulation of the CR array is designed and implemented. This approach with enhanced security, large information capacity, and high-level integration at a deep subwavelength scale may find applications in photonic devices and emerging areas in quantum information technologies.
Live imaging of the extracellular matrix with a glycan-binding fluorophore
All multicellular systems produce and dynamically regulate extracellular matrices (ECMs) that play essential roles in both biochemical and mechanical signaling. Though the spatial arrangement of these extracellular assemblies is critical to their biological functions, visualization of ECM structure is challenging, in part because the biomolecules that compose the ECM are difficult to fluorescently label individually and collectively. Here, we present a cell-impermeable small-molecule fluorophore, termed Rhobo6, that turns on and red shifts upon reversible binding to glycans. Given that most ECM components are densely glycosylated, the dye enables wash-free visualization of ECM, in systems ranging from in vitro substrates to in vivo mouse mammary tumors. Relative to existing techniques, Rhobo6 provides a broad substrate profile, superior tissue penetration, non-perturbative labeling, and negligible photobleaching. This work establishes a straightforward method for imaging the distribution of ECM in live tissues and organisms, lowering barriers for investigation of extracellular biology.
Universal conservation laws of the wave-particle-entanglement triad: theory and experiment
When observed, a quantum system exhibits either wave-like or particle-like properties, depending on how it is measured. However, this duality is affected by the entanglement of the system with its quantum memory, raising a fundamental question: how are wave–particle duality and entanglement related? Here, we broaden the scope of wave–particle duality to include entanglement, introduce universal conservation laws for the wave–particle–entanglement triad, and perform demonstrations on silicon–integrated nanophotonic quantum chips. Our experiments not only mark the first confirmation of universal conservation laws but also highlight the potential of integrated photonics for exploring complex quantum phenomena in high-dimensional systems.
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